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EnglishA ruthenium-catalysed dehy drogenativecross-coupling of primary alcohols and imines inthe presence of TFA provided a library of different-ly substituted quinolines. Imines can be prepared insitu from various anilines and several benzyl alco-hols using a ruthenium-catalysed hydrogen-transferprocedure. Without changing the catalyst, quino-lines can be obtained in moderate to good yields byadding various primary alcohols in the presence ofTFA (30 mol%) via a “telescopic” protocol. Theuse of alcohols, the absence of strong oxidants andthe diversity of potential starting materials makethis modern version of the Skraup reaction superi orto most of the conventional quinoline syntheses.
A mild and efficient synthesis of substituted quinolines via a cross-dehydrogenative coupling of (bio)available alcohols and aminoarenes / Mura, M G; Rajamäki, S; De Luca, L; Cini, E; Porcheddu, A. - In: ADVANCED SYNTHESIS & CATALYSIS. - ISSN 1615-4150. - 357:2-3(2015), pp. 576-582.
| Titolo: | A mild and efficient synthesis of substituted quinolines via a cross-dehydrogenative coupling of (bio)available alcohols and aminoarenes |
| Autori: | |
| Data di pubblicazione: | 2015 |
| Rivista: | |
| Citazione: | A mild and efficient synthesis of substituted quinolines via a cross-dehydrogenative coupling of (bio)available alcohols and aminoarenes / Mura, M G; Rajamäki, S; De Luca, L; Cini, E; Porcheddu, A. - In: ADVANCED SYNTHESIS & CATALYSIS. - ISSN 1615-4150. - 357:2-3(2015), pp. 576-582. |
| Handle: | http://hdl.handle.net/11584/143947 |
| Tipologia: | 1.1 Articolo in rivista |
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http://hdl.handle.net/11584/143947
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